Artículo
H2-rich syngas production from biogas reforming: overcoming coking and sintering using bimetallic Ni-based catalysts
Autor/es | Carrasco Ruiz, Sergio
Zhang, Qi Gándara Loe, Jesús Pastor Pérez, Laura Odriozola Gordón, José Antonio Ramírez Reina, Tomás Bobadilla Baladrón, Luis Francisco |
Departamento | Universidad de Sevilla. Departamento de Química Inorgánica |
Fecha de publicación | 2023-08-22 |
Fecha de depósito | 2023-10-31 |
Publicado en |
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Resumen | Dry reforming of methane is a very appealing catalytic route biogas (mainly composed by greenhouse gases: carbon dioxide and methane) conversion into added value syngas, which could be further upgraded to produce liquid ... Dry reforming of methane is a very appealing catalytic route biogas (mainly composed by greenhouse gases: carbon dioxide and methane) conversion into added value syngas, which could be further upgraded to produce liquid fuels and added value chemicals. However, the major culprits of this reaction are coking and active phase sintering that result in catalysts deactivation. Herein we have developed a highly stable bimetallic Ni–Rh catalyst supported on mixed CeO2–Al2O3 oxide using low-noble metal loadings. The addition of small amounts of rhodium to nickel catalysts prevents coke formation and improves sintering resistance, achieving high conversions over extended reaction times hence resulting in promising catalysts for biogas upgrading. © 2023 The Author(s) |
Agencias financiadoras | Ministerio de Ciencia e Innovación (MICIN). España European Commission (EC) |
Identificador del proyecto | PLEC2021-008086
RYC2018- 024387-I PID2019-108502RJ-I00 101008058 |
Cita | Carrasco Ruiz, S., Zhang, Q., Gándara Loe, J., Pastor Pérez, L., Odriozola Gordón, J.A., Ramírez Reina, T. y Bobadilla Baladrón, L.F. (2023). H2-rich syngas production from biogas reforming: overcoming coking and sintering using bimetallic Ni-based catalysts. International Journal of Hydrogen Energy, 48 (72), 27907-27917. https://doi.org/10.1016/j.ijhydene.2023.03.301. |
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