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Versatile Ni-Ru catalysts for gas phase CO2 conversion: Bringing closer dry reforming, reverse water gas shift and methanation to enable end-products flexibility
dc.creator | Merkouri, Loukia Pantzechroula | es |
dc.creator | Le Saché, Estelle | es |
dc.creator | Pastor Pérez, Laura | es |
dc.creator | Duyar, Melis S. | es |
dc.creator | Ramírez Reina, Tomás | es |
dc.date.accessioned | 2022-09-16T07:47:23Z | |
dc.date.available | 2022-09-16T07:47:23Z | |
dc.date.issued | 2022 | |
dc.identifier.citation | Merkouri, L.P., Le Saché, E., Pastor Pérez, L., Duyar, M.S. y Ramírez Reina, T. (2022). Versatile Ni-Ru catalysts for gas phase CO2 conversion: Bringing closer dry reforming, reverse water gas shift and methanation to enable end-products flexibility. Fuel, 315, 123097. | |
dc.identifier.issn | 1873-7153 | es |
dc.identifier.uri | https://hdl.handle.net/11441/137123 | |
dc.description.abstract | Advanced catalytic materials able to catalyse more than one reaction efficiently are needed within the CO2 utilisation schemes to benefit from end-products flexibility. In this study, the combination of Ni and Ru (15 and 1 wt%, respectively) was tested in three reactions, i.e. dry reforming of methane (DRM), reverse water–gas shift (RWGS) and CO2 methanation. A stability experiment with one cycle of CO2 methanation-RWGS-DRM was carried out. Outstanding stability was revealed for the CO2 hydrogenation reactions and as regards the DRM, coke formation started after 10 h on stream. Overall, this research showcases that a multicomponent Ni-Ru/CeO2-Al2O3 catalyst is an unprecedent versatile system for gas phase CO2 recycling. Beyond its excellent performance, our switchable catalyst allows a fine control of end-products selectivity. | es |
dc.format | application/pdf | es |
dc.format.extent | 10 p. | es |
dc.language.iso | eng | es |
dc.publisher | Elsevier | es |
dc.relation.ispartof | Fuel, 315, 123097. | |
dc.rights | Attribution-NonCommercial-NoDerivatives 4.0 Internacional | * |
dc.rights.uri | http://creativecommons.org/licenses/by-nc-nd/4.0/ | * |
dc.title | Versatile Ni-Ru catalysts for gas phase CO2 conversion: Bringing closer dry reforming, reverse water gas shift and methanation to enable end-products flexibility | es |
dc.type | info:eu-repo/semantics/article | es |
dcterms.identifier | https://ror.org/03yxnpp24 | |
dc.type.version | info:eu-repo/semantics/publishedVersion | es |
dc.rights.accessRights | info:eu-repo/semantics/openAccess | es |
dc.contributor.affiliation | Universidad de Sevilla. Departamento de Química Inorgánica | es |
dc.relation.publisherversion | https://doi.org/10.1016/j.fuel.2021.123097 | es |
dc.identifier.doi | 10.1016/j.fuel.2021.123097 | es |
dc.journaltitle | Fuel | es |
dc.publication.volumen | 315 | es |
dc.publication.endPage | 123097 | es |
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