Purcell Enhancement and Wavelength Shift of Emitted Light by CsPbI3 Perovskite Nanocrystals Coupled to Hyperbolic Metamaterials

Adl, Hamid Pashaei; Gorji, Setatira; Habil, Mojtaba Karimi; Suárez, Isaac; Chirvony, Vladimir S.; Gualdrón-Reyes, Andrés F.; Mora-Seró, Iván; Valencia Liñán, Luisa María; Mata, María de la; Hernández-Saz, Jesús; Molina, Sergio I.; Zapata-Rodríguez, Carlos J.; Martínez-Pastor, Juan P.

doi:10.1021/acsphotonics.0c01219

Artículo

dc.creator	Adl, Hamid Pashaei	es
dc.creator	Gorji, Setatira	es
dc.creator	Habil, Mojtaba Karimi	es
dc.creator	Suárez, Isaac	es
dc.creator	Chirvony, Vladimir S.	es
dc.creator	Gualdrón-Reyes, Andrés F.	es
dc.creator	Mora-Seró, Iván	es
dc.creator	Valencia Liñán, Luisa María	es
dc.creator	Mata, María de la	es
dc.creator	Hernández-Saz, Jesús	es
dc.creator	Molina, Sergio I.	es
dc.creator	Zapata-Rodríguez, Carlos J.	es
dc.creator	Martínez-Pastor, Juan P.	es
dc.date.accessioned	2020-12-10T11:20:39Z
dc.date.available	2020-12-10T11:20:39Z
dc.date.issued	2020
dc.identifier.citation	Adl, H.P., Gorji, S., Habil, M.K., Suárez, I., Chirvony, V.S., Gualdrón-Reyes, A.F.,...,Martínez-Pastor, J.P. (2020). Purcell Enhancement and Wavelength Shift of Emitted Light by CsPbI3 Perovskite Nanocrystals Coupled to Hyperbolic Metamaterials. ACS Photonics, 7 (11), 3152-3160.
dc.identifier.issn	2330-4022	es
dc.identifier.uri	https://hdl.handle.net/11441/103109
dc.description	"This is an open access article published under an ACS AuthorChoice License, which permits copying and redistribution of the article or any adaptations for non-commercial purposes". http://pubs.acs.org/page/policy/authorchoice_termsofuse.html	es
dc.description.abstract	Manipulation of the exciton emission rate in nanocrystals of lead halide perovskites (LHPs) was demonstrated by means of coupling of excitons with a hyperbolic metamaterial (HMM) consisting of alternating thin metal (Ag) and dielectric (LiF) layers. Such a coupling is found to induce an increase of the exciton radiative recombination rate by more than a factor of three due to the Purcell effect when the distance between the quantum emitter and HMM is nominally as small as 10 nm, which coincides well with the results of our theoretical analysis. Besides, an effect of the coupling-induced long wavelength shift of the exciton emission spectrum is detected and modeled. These results can be of interest for quantum information applications of single emitters on the basis of perovskite nanocrystals with high photon emission rates.	es
dc.description.sponsorship	Ministerio de Economía y Competitividad TEC2017-86102-C2-1-R,TEC2017-86102-C2-2-R	es
dc.description.sponsorship	Ministerio de Ciencia e Innovación IJCI-2017-31507	es
dc.description.sponsorship	Fondos FEDER FEDER-UCA18-106586,TEP946	es
dc.description.sponsorship	European Research Council 724424-No-LIMIT	es
dc.format	application/pdf	es
dc.format.extent	9 p.	es
dc.language.iso	eng	es
dc.publisher	ACS Publications	es
dc.relation.ispartof	ACS Photonics, 7 (11), 3152-3160.
dc.rights	Attribution-NonCommercial-NoDerivatives 4.0 Internacional	*
dc.rights.uri	http://creativecommons.org/licenses/by-nc-nd/4.0/	*
dc.subject	Lead halide perovskites	es
dc.subject	Perovskite nanocrystals	es
dc.subject	Photonics	es
dc.subject	Hyperbolic metamaterials (HMMs)	es
dc.subject	Light−matter interaction	es
dc.subject	Purcell factor	es
dc.title	Purcell Enhancement and Wavelength Shift of Emitted Light by CsPbI3 Perovskite Nanocrystals Coupled to Hyperbolic Metamaterials	es
dc.type	info:eu-repo/semantics/article	es
dcterms.identifier	https://ror.org/03yxnpp24
dc.type.version	info:eu-repo/semantics/publishedVersion	es
dc.rights.accessRights	info:eu-repo/semantics/embargoedAccess	es
dc.contributor.affiliation	Universidad de Sevilla. Departamento de Ingeniería y Ciencia de los Materiales y del Transporte	es
dc.relation.projectID	TEC2017-86102-C2-1-R	es
dc.relation.projectID	TEC2017-86102-C2-2-R	es
dc.relation.projectID	IJCI-2017-31507	es
dc.relation.projectID	FEDER-UCA18-106586,TEP946	es
dc.relation.projectID	724424-No-LIMIT	es
dc.date.embargoEndDate	2021-12-01
dc.relation.publisherversion	https://pubs.acs.org/doi/full/10.1021/acsphotonics.0c01219	es
dc.identifier.doi	10.1021/acsphotonics.0c01219	es
dc.journaltitle	ACS Photonics	es
dc.publication.volumen	7	es
dc.publication.issue	11	es
dc.publication.initialPage	3152	es
dc.publication.endPage	3160	es

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