Artículo
Highly Dispersed Rh Single Atoms over Graphitic Carbon Nitride as a Robust Catalyst for the Hydroformylation Reaction
Autor/es | Jurado, Lole
Esvan, Jerome Luque Álvarez, Ligia Amelia Bobadilla Baladrón, Luis Francisco Odriozola Gordón, José Antonio Posada Pérez, Sergio Poater, Albert Comas Vives, Aleix Axet, M. Rosa |
Departamento | Universidad de Sevilla. Departamento de Química Inorgánica |
Fecha de publicación | 2023 |
Fecha de depósito | 2023-09-15 |
Publicado en |
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Resumen | Rhodium-catalysed hydroformylation, effective tool in bulk and fine-chemical synthesis, predominantly uses soluble metal complexes. For that reason, the metal leaching and the catalyst recycling are still the major drawbacks ... Rhodium-catalysed hydroformylation, effective tool in bulk and fine-chemical synthesis, predominantly uses soluble metal complexes. For that reason, the metal leaching and the catalyst recycling are still the major drawbacks of this process. Single-atom catalysts have emerged as a powerful tool to combine the advantages of both homogeneous and heterogeneous catalysts. Since using an appropriate support material is key to create stable, finely dispersed, single-atom catalysts, here we show that Rh atoms anchored on graphitic carbon nitride are robust catalysts for the hydroformylation reaction of styrene. |
Agencias financiadoras | Ministerio de Ciencia e Innovación (MICIN). España European Commission. Fondo Social Europeo (FSO) European Union (UE) |
Identificador del proyecto | PID2021-127423NB-I00
PGC2018-100818-A-I00 RyC-2016-19930 H2020-MSCA-IF-2020-101020330 FJC2019-039623-I |
Cita | Jurado, L., Esvan, J., Luque Álvarez, L.A., Bobadilla Baladrón, L.F., Odriozola Gordón, J.A., Posada Pérez, S.,...,Axet, M.R. (2023). Highly Dispersed Rh Single Atoms over Graphitic Carbon Nitride as a Robust Catalyst for the Hydroformylation Reaction. Catalysis Science and Technology, 13 (5), 1425-1436. https://doi.org/DOI: 10.1039/d2cy02094g. |
Ficheros | Tamaño | Formato | Ver | Descripción |
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Highly dispersed Rh.pdf | 2.587Mb | [PDF] | Ver/ | |